| 151 | 1966 | Walter Matthau - The Fortune Cookie - "Willie Gingrich" |
| 152 | 1966 | Mako - The Sand Pebbles - "Po-han" |
| 153 | 1966 | James Mason - Georgy Girl - "James Leamington" |
| 154 | 1966 | George Segal - Who's Afraid of Virginia Woolf? - "Nick" |
| 155 | 1966 | Robert Shaw - A Man for All Seasons - Henry VIII |
| 156 | 1967 | George Kennedy - Cool Hand Luke - "Dragline" |
| 157 | 1967 | John Cassavetes - The Dirty Dozen - "Victor P. Franko" |
| 158 | 1967 | Gene Hackman - Bonnie and Clyde - Buck Barrow |
| 159 | 1967 | Cecil Kellaway - Guess Who's Coming to Dinner - "Monsignor Mike Ryan" |
| 160 | 1967 | Michael J. Pollard - Bonnie and Clyde - "C.W. Moss" |
| 161 | 1968 | Jack Albertson - The Subject Was Roses - "John Cleary" |
| 162 | 1968 | Seymour Cassel - Faces - "Chet" |
| 163 | 1968 | Daniel Massey - Star! - Noel Coward |
| 164 | 1968 | Jack Wild - Oliver! - "The Artful Dodger" |
| 165 | 1968 | Gene Wilder - The Producers - "Leo Bloom" |
| 166 | 1969 | Gig Young - They Shoot Horses, Don't They? - "Rocky" |
| 167 | 1969 | Rupert Crosse - The Reivers - "Ned" |
| 168 | 1969 | Elliott Gould - Bob & Carol & Ted & Alice - "Ted Henderson" |
| 169 | 1969 | Jack Nicholson - E -y Rider - "George Hanson" |
| 170 | 1969 | Anthony Quayle - Anne of the Thousand Days - Cardinal Wolsey |
| 171 | 1970 | John Mills - Ryan's Daughter - "Michael" |
| 172 | 1970 | Richard S. Castellano - Lovers and Other Strangers - "Frank Vecchio" |
| 173 | 1970 | Dan George - Little Big Man - "Old Lodge Skins" |
| 174 | 1970 | Gene Hackman - I Never Sang for My Father - "Gene Garrison" |
| 175 | 1970 | John Marley - Love Story - "Phil Cavalleri" |
| 176 | 1971 | Ben Johnson - The Last Picture Show - "Sam the Lion" |
| 177 | 1971 | Jeff Bridges - The Last Picture Show - "Duane Jackson" |
| 178 | 1971 | Leonard Frey - Fiddler on the Roof - "Motel Kamzoil" |
| 179 | 1971 | Richard Jaeckel - Sometimes a Great Notion - "Joe Ben Stamper" |
| 180 | 1971 | Roy Scheider - The French Connection - "Detective Buddy 'Cloudy' Russo" |